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Abstract

A modified approach to equilibrium modelling of coal gasification is presented, based on global thermodynamic analysis of both homogeneous and heterogeneous reactions occurring during a gasification process conducted in a circulating fluid bed reactor. The model is based on large-scale experiments (ca. 200 kg/h) with air used as a gasification agent and introduces empirical modifications governing the quasi-equilibrium state of two reactions: water-gas shift and Boudouard reaction. The model predicts the formation of the eight key gaseous species: CO, CO2, H2O, H2, H2S, N2, COS and CH4, volatile hydrocarbons represented by propane and benzene, tar represented by naphthalene, and char containing the five elements C, H, O, N, S and inorganic matter.
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Abstract

The subject of the CFD analysis presented in this paper is the process of biomass indirect co-firing carried out in a system composed of a stoker-fired furnace coupled with a gasification reactor. The installation is characterised by its compact structure, which makes it possible to minimise heat losses to the environment and enhance the physical enthalpy of the oxidising agent – flue gases – having a favourable chemical composition with oxygen and water vapour. The test results provided tools for modelling of biomass thermal processing using a non-standard oxidiser in the form of flue gases. The obtained models were used to optimise the indirect co-combustion process to reduce emissions. An overall effect of co-combustion of gas from biomass gasification in the stoker furnace is the substantial reduction in NO emissions by about 22%.
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